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The Golden Age of Thermally Activated Delayed Fluorescence Materials: Design and Exploitation

Marques dos Santos, John; Hall, David; Basumatary, Biju; Bryden, Megan; Chen, Dongyang; Choudhary, Praveen; Comerford, Thomas; Crovini, Ettore; Danos, Andrew; De, Joydip; Diesing, Stefan; Fatahi, Mahni; Griffin, Maire; Kumar Gupta, Abhishek; Hafeez, Hassan; Hämmerling, Lea; Hanover, Emily; Haug, Janine; Heil, Tabea; Karthik, Durai; Kumar, Shiv; Lee, Oliver; Li, Haoyang; Lucas, Fabien; Frank Ross Mackenzie, Campbell; Mariko, Aminata; Matulaitis, Tomas; Millward, Francis; Olivier, Yoann; Qi, Quan; Samuel, Ifor D.W.; Sharma, Nidhi; Si, Changfeng; Spierling, Leander; Sudhakar, Pagidi; Sun, Dianming; Tankelevičiūtė, Eglė; Duarte Tonet, Michele; Wang, Jingxiang; Wang, Tao; Wu, Sen; Xu, Yan; Zhang, Le; Zysman-Colman, Eli

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Authors

John Marques dos Santos

David Hall

Biju Basumatary

Megan Bryden

Dongyang Chen

Praveen Choudhary

Thomas Comerford

Ettore Crovini

Joydip De

Stefan Diesing

Mahni Fatahi

Maire Griffin

Abhishek Kumar Gupta

Hassan Hafeez

Lea Hämmerling

Emily Hanover

Janine Haug

Tabea Heil

Durai Karthik

Shiv Kumar

Oliver Lee

Haoyang Li

Fabien Lucas

Campbell Frank Ross Mackenzie

Aminata Mariko

Tomas Matulaitis

Francis Millward

Yoann Olivier

Quan Qi

Ifor D.W. Samuel

Nidhi Sharma

Changfeng Si

Leander Spierling

Pagidi Sudhakar

Dianming Sun

Eglė Tankelevičiūtė

Michele Duarte Tonet

Jingxiang Wang

Tao Wang

Sen Wu

Yan Xu

Le Zhang

Eli Zysman-Colman



Abstract

Since the seminal report by Adachi and co-workers in 2012, there has been a veritable explosion of interest in the design of thermally activated delayed fluorescence (TADF) compounds, particularly as emitters for organic light-emitting diodes (OLEDs). With rapid advancements and innovation in materials design, the efficiencies of TADF OLEDs for each of the primary color points as well as for white devices now rival those of state-of-the-art phosphorescent emitters. Beyond electroluminescent devices, TADF compounds have also found increasing utility and applications in numerous related fields, from photocatalysis, to sensing, to imaging and beyond. Following from our previous review in 2017 ( Adv. Mater. 2017, 1605444 ), we here comprehensively document subsequent advances made in TADF materials design and their uses from 2017–2022. Correlations highlighted between structure and properties as well as detailed comparisons and analyses should assist future TADF materials development. The necessarily broadened breadth and scope of this review attests to the bustling activity in this field. We note that the rapidly expanding and accelerating research activity in TADF material development is indicative of a field that has reached adolescence, with an exciting maturity still yet to come.

Citation

Marques dos Santos, J., Hall, D., Basumatary, B., Bryden, M., Chen, D., Choudhary, P., Comerford, T., Crovini, E., Danos, A., De, J., Diesing, S., Fatahi, M., Griffin, M., Kumar Gupta, A., Hafeez, H., Hämmerling, L., Hanover, E., Haug, J., Heil, T., Karthik, D., …Zysman-Colman, E. (2024). The Golden Age of Thermally Activated Delayed Fluorescence Materials: Design and Exploitation. Chemical Reviews, 124(24), 13736-14110. https://doi.org/10.1021/acs.chemrev.3c00755

Journal Article Type Review
Acceptance Date Jun 4, 2024
Online Publication Date Dec 12, 2024
Publication Date Dec 25, 2024
Deposit Date Jun 5, 2024
Publicly Available Date Dec 13, 2024
Journal Chemical Reviews
Print ISSN 0009-2665
Electronic ISSN 1520-6890
Publisher American Chemical Society
Peer Reviewed Peer Reviewed
Volume 124
Issue 24
Pages 13736-14110
DOI https://doi.org/10.1021/acs.chemrev.3c00755
Public URL https://durham-repository.worktribe.com/output/2473564

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