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Ratchet behaviour of polarons in molecular chains

Brizhik, L.S.; Eremko, A.A.; Piette, B.M.A.G.; Zakrzewski, W.J.

Authors

L.S. Brizhik

A.A. Eremko

W.J. Zakrzewski



Abstract

We study the ratchet behaviour of polarons in diatomic molecular chains under the influence of an external electromagnetic field which is periodic in time. We show that in asymmetric chains a harmonic unbiased field causes a drift of polarons. This phenomenon has a threshold with respect to the intensity and the frequency of the field. In spatially symmetric chains a harmonic periodic electric field generates oscillations of polarons but does not result in their movement. The polaron drift current can be induced in symmetric chains by a time periodic asymmetric external field. This complex dynamics of polarons is generated by the interplay between the Peierls–Nabarro barrier and dissipative effects in the chains.

Citation

Brizhik, L., Eremko, A., Piette, B., & Zakrzewski, W. (2008). Ratchet behaviour of polarons in molecular chains. Journal of Physics: Condensed Matter, 20(25), https://doi.org/10.1088/0953-8984/20/25/255242

Journal Article Type Other
Publication Date 2008
Deposit Date Nov 22, 2010
Journal Journal of Physics: Condensed Matter
Print ISSN 0953-8984
Electronic ISSN 1361-648X
Publisher IOP Publishing
Peer Reviewed Peer Reviewed
Volume 20
Issue 25
DOI https://doi.org/10.1088/0953-8984/20/25/255242
Keywords Self-trapped or small polarons, Bipolarons
Public URL https://durham-repository.worktribe.com/output/1617992
Publisher URL http://iopscience.iop.org/0953-8984/20/25/255242