Skip to main content

Research Repository

Advanced Search

Outputs (120)

Origin of Magnetic Ordering in a Structurally Perfect Quantum Kagome Antiferromagnet (2020)
Journal Article
Arh, T., Gomilšek, M., Prelovšek, P., Pregelj, M., Klanjšek, M., Ozarowski, A., Clark, S., Lancaster, T., Sun, W., Mi, J.-X., & Zorko, A. (2020). Origin of Magnetic Ordering in a Structurally Perfect Quantum Kagome Antiferromagnet. Physical Review Letters, 125(2), Article 027203. https://doi.org/10.1103/physrevlett.125.027203

The ground state of the simple Heisenberg nearest-neighbor quantum kagome antiferromagnetic model is a magnetically disordered spin liquid, yet various perturbations may lead to fundamentally different states. Here we disclose the origin of magnetic... Read More about Origin of Magnetic Ordering in a Structurally Perfect Quantum Kagome Antiferromagnet.

Magnetism and Néel skyrmion dynamics in GaV4S8−ySey (2020)
Journal Article
Hicken, T., Holt, S., Franke, K., Hawkhead, Z., Štefančič, A., Wilson, M., Gomilšek, M., Huddart, B., Clark, S., Lees, M., Pratt, F., Blundell, S., Balakrishnan, G., & Lancaster, T. (2020). Magnetism and Néel skyrmion dynamics in GaV4S8−ySey. Physical Review Research, 2(3), Article 032001. https://doi.org/10.1103/physrevresearch.2.032001

We present an investigation of the influence of low levels of chemical substitution on the magnetic ground state and Néel skyrmion lattice (SkL) state in GaV4S8−ySey, where y=0,0.1,7.9, and 8. Muon-spin spectroscopy (μSR) measurements on y=0 and 0.1... Read More about Magnetism and Néel skyrmion dynamics in GaV4S8−ySey.

Establishing magneto-structural relationships in the solid solutions of the skyrmion hosting family of materials: GaV4S8−ySey (2020)
Journal Article
Štefančič, A., Holt, S. J., Lees, M. R., Ritter, C., Gutmann, M. J., Lancaster, T., & Balakrishnan, G. (2020). Establishing magneto-structural relationships in the solid solutions of the skyrmion hosting family of materials: GaV4S8−ySey. Scientific Reports, 10(1), Article 9813. https://doi.org/10.1038/s41598-020-65676-9

The GaV4S8−ySey (y = 0 to 8) family of materials have been synthesized in both polycrystalline and single crystal form, and their structural and magnetic properties thoroughly investigated. Each of these materials crystallizes in the Fˉ 43m space gro... Read More about Establishing magneto-structural relationships in the solid solutions of the skyrmion hosting family of materials: GaV4S8−ySey.

Near-ideal molecule-based Haldane spin chain (2020)
Journal Article
Williams, R. C., Blackmore, W. J., Curley, S. P., Lees, M. R., Birnbaum, S. M., Singleton, J., Huddart, B. M., Hicken, T. J., Lancaster, T., Blundell, S. J., Xiao, F., Ozarowski, A., Pratt, F. L., Voneshen, D. J., Guguchia, Z., Baines, C., Schlueter, J. A., Villa, D. Y., Manson, J. L., & Goddard, P. A. (2020). Near-ideal molecule-based Haldane spin chain. Physical Review Research, 2(1), Article 013082. https://doi.org/10.1103/physrevresearch.2.013082

The molecular coordination complex NiI2 (3, 5-lut)4 [where (3,5-lut) = (3,5-lutidine) = (C7H9N)] has been synthesized and characterized by several techniques including synchrotron x-ray diffraction, electron-spin resonance, superconducting quantum in... Read More about Near-ideal molecule-based Haldane spin chain.

Enhancing easy-plane anisotropy in bespoke Ni(II) quantum magnets (2020)
Journal Article
Manson, J. L., Manson, Z. E., Sargent, A., Villa, D. Y., Etten, N. L., Blackmore, W. J., Curley, S. P., Williams, R. C., Brambleby, J., Goddard, P. A., Ozarowski, A., Wilson, M. N., Huddart, B. M., Lancaster, T., Johnson, R. D., Blundell, S. J., Bendix, J., Wheeler, K. A., Lapidus, S. H., Xiao, F., …Singleton, J. (2020). Enhancing easy-plane anisotropy in bespoke Ni(II) quantum magnets. Polyhedron, 180, Article 114379. https://doi.org/10.1016/j.poly.2020.114379

We examine the crystal structures and magnetic properties of several S = 1 Ni(II) coordination compounds, molecules and polymers, that include the bridging ligands HF2-, AF62- (A = Ti, Zr) and pyrazine or non-bridging ligands F-, SiF62-, glycine, H2O... Read More about Enhancing easy-plane anisotropy in bespoke Ni(II) quantum magnets.

Investigating the magnetic ground state of the skyrmion host material Cu2OSeO3 using long-wavelength neutron diffraction (2019)
Journal Article
Franke, K., Dean, P., Hatnean, M. C., Birch, M., Khalyavin, D., Manuel, P., Lancaster, T., Balakrishnan, G., & Hatton, P. (2019). Investigating the magnetic ground state of the skyrmion host material Cu2OSeO3 using long-wavelength neutron diffraction. AIP Advances, 9(12), Article 125228. https://doi.org/10.1063/1.5129400

We present long-wavelength neutron diffraction data measured on both single crystal and polycrystalline samples of the skyrmion host material Cu2OSeO3. We observe magnetic satellites around the (01⎯⎯1) diffraction peak not accessible to other techniq... Read More about Investigating the magnetic ground state of the skyrmion host material Cu2OSeO3 using long-wavelength neutron diffraction.

Determining the anisotropy and exchange parameters of polycrystalline spin-1 magnets (2019)
Journal Article
Blackmore, W., Brambleby, J., Lancaster, T., Clark, S., Johnson, R., Singleton, J., Ozarowski, A., Schlueter, J., Chen, Y.-S., Arif, A., Lapidus, S., Xiao, F., Williams, R., Blundell, S., Pearce, M., Lees, M., Manuel, P., Villa, D., Villa, J., Manson, J., & Goddard, P. (2019). Determining the anisotropy and exchange parameters of polycrystalline spin-1 magnets. New Journal of Physics, 21(9), https://doi.org/10.1088/1367-2630/ab3dba

Although low-dimensional S = 1 antiferromagnets remain of great interest, difficulty in obtaining highquality single crystals of the newest materials hinders experimental research in this area. Polycrystalline samples are more readily produced, but t... Read More about Determining the anisotropy and exchange parameters of polycrystalline spin-1 magnets.

Increased lifetime of metastable skyrmions by controlled doping (2019)
Journal Article
Birch, M., Takagi, R., Seki, S., Wilson, M., Kagawa, F., Štefančič, A., Balakrishnan, G., Fan, R., Steadman, P., Ottley, C., Crisanti, M., Cubitt, R., Lancaster, T., Tokura, Y., & Hatton, P. (2019). Increased lifetime of metastable skyrmions by controlled doping. Physical review B - Condensed Matter and Materials Physics, 100(1), Article 014425. https://doi.org/10.1103/physrevb.100.014425

Previous observations of metastable magnetic skyrmions have shown that close to the equilibrium pocket the metastable state has a short lifetime, and therefore, rapid cooling is required to generate a significant skyrmion population at low temperatur... Read More about Increased lifetime of metastable skyrmions by controlled doping.

Probing magnetic order and disorder in the one-dimensional molecular spin chains CuF2(pyz) and [Ln(hfac)3(boaDTDA)] n (Ln  =  Sm, La) using implanted muons (2019)
Journal Article
Lancaster, T., Huddart, B., Williams, R., Xiao, F., Franke, K., Baker, P., Pratt, F., Blundell, S., Schlueter, J., Mills, M., Maahs, A., & Preuss, K. (2019). Probing magnetic order and disorder in the one-dimensional molecular spin chains CuF2(pyz) and [Ln(hfac)3(boaDTDA)] n (Ln  =  Sm, La) using implanted muons. Journal of Physics: Condensed Matter, 31(39), Article 394002. https://doi.org/10.1088/1361-648x/ab2cb6

We present the results of muon-spin relaxation (SR) measurements on antiferromagnetic and ferromagnetic spin chains. In antiferromagnetic CuF2(pyz) we identify a transition to long range magnetic order taking place at K, allowing us to estimate a rat... Read More about Probing magnetic order and disorder in the one-dimensional molecular spin chains CuF2(pyz) and [Ln(hfac)3(boaDTDA)] n (Ln  =  Sm, La) using implanted muons.