All Outputs (7)

Charged Particle Imaging of the Deprotonated Octatrienoic Acid Anion: Evidence for a Photoinduced Cyclization Reaction (2016)
Journal Article
West, C., Bull, J., & Verlet, J. (2016). Charged Particle Imaging of the Deprotonated Octatrienoic Acid Anion: Evidence for a Photoinduced Cyclization Reaction. Journal of Physical Chemistry Letters, 7(22), 4635-4640. https://doi.org/10.1021/acs.jpclett.6b02302

Photoelectron spectroscopy of the deprotonated octatrienoic acid anion, [C7H9–CO2]−, shows the formation of [C7H9]− and loss of H– at hν = 4.13 eV. Using velocity map imaging, the H– fragment was characterized to have a Boltzmann-like kinetic energy... Read More about Charged Particle Imaging of the Deprotonated Octatrienoic Acid Anion: Evidence for a Photoinduced Cyclization Reaction.

Charge Transfer to Solvent Dynamics at the Ambient Water/Air Interface (2016)
Journal Article
Nowakowski, P., Woods, D., & Verlet, J. (2016). Charge Transfer to Solvent Dynamics at the Ambient Water/Air Interface. Journal of Physical Chemistry Letters, 7(20), 4079-4085. https://doi.org/10.1021/acs.jpclett.6b01985

Electron-transfer reactions at ambient aqueous interfaces represent one of the most fundamental and ubiquitous chemical reactions. Here the dynamics of the charge transfer to solvent (CTTS) reaction from iodide was probed at the ambient water/air int... Read More about Charge Transfer to Solvent Dynamics at the Ambient Water/Air Interface.

Plasma–liquid interactions: a review and roadmap (2016)
Journal Article
Bruggeman, P., Kushner, M., Locke, B., Gardeniers, J., Graham, W., Graves, D., …Zvereva, G. (2016). Plasma–liquid interactions: a review and roadmap. Plasma Sources Science and Technology, 25(5), Article 053002. https://doi.org/10.1088/0963-0252/25/5/053002

Plasma–liquid interactions represent a growing interdisciplinary area of research involving plasma science, fluid dynamics, heat and mass transfer, photolysis, multiphase chemistry and aerosol science. This review provides an assessment of the state-... Read More about Plasma–liquid interactions: a review and roadmap.

Ultrafast dynamics of temporary anions probed through the prism of photodetachment (2016)
Journal Article
Anstöter, C., Bull, J., & Verlet, J. (2016). Ultrafast dynamics of temporary anions probed through the prism of photodetachment. International Reviews in Physical Chemistry, 35(4), 509-538. https://doi.org/10.1080/0144235x.2016.1203522

The recently developed method of frequency-, angle-, and time-resolved photoelectron imaging (FAT-PI) applied to the study of the dynamics of resonances of open-shell anions is reviewed. The basic principles of the method and its experimental realisa... Read More about Ultrafast dynamics of temporary anions probed through the prism of photodetachment.

The Vitamin E Radical Probed by Anion Photoelectron Imaging (2016)
Journal Article
Anstöter, C., West, C., Bull, J., & Verlet, J. (2016). The Vitamin E Radical Probed by Anion Photoelectron Imaging. Journal of Physical Chemistry B (Soft Condensed Matter and Biophysical Chemistry), 120(29), 7108-7113. https://doi.org/10.1021/acs.jpcb.6b05271

The biological antioxidant activity of vitamin E has been related to the stability of the tocopheroxyl radical. Using anion photoelectron imaging and electronic structure calculations, the four tocopheroxyl components of vitamin E have been studied i... Read More about The Vitamin E Radical Probed by Anion Photoelectron Imaging.

Ultrafast dynamics of formation and autodetachment of a dipole-bound state in an open-shell π-stacked dimer anion (2016)
Journal Article
Bull, J., West, C., & Verlet, J. (2016). Ultrafast dynamics of formation and autodetachment of a dipole-bound state in an open-shell π-stacked dimer anion. Chemical Science, 7(8), 5352-5361. https://doi.org/10.1039/c6sc01062h

Isolated π-stacked dimer radical anions present the simplest model of an excess electron in a π-stacked environment. Here, frequency-, angle-, and time-resolved photoelectron imaging together with electronic structure calculations have been used to c... Read More about Ultrafast dynamics of formation and autodetachment of a dipole-bound state in an open-shell π-stacked dimer anion.

Gas-Phase Femtosecond Particle Spectroscopy: A Bottom-Up Approach to Nucleotide Dynamics (2016)
Journal Article
Stavros, V., & Verlet, J. (2016). Gas-Phase Femtosecond Particle Spectroscopy: A Bottom-Up Approach to Nucleotide Dynamics. Annual Review of Physical Chemistry, 67(1), 211-232. https://doi.org/10.1146/annurev-physchem-040215-112428

We summarize how gas-phase ultrafast charged-particle spectroscopy has been used to provide an understanding of the photophysics of DNA building blocks. We focus on adenine and discuss how, following UV excitation, specific interactions determine the... Read More about Gas-Phase Femtosecond Particle Spectroscopy: A Bottom-Up Approach to Nucleotide Dynamics.